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Hill country by Barcelona

We are traveling to Spain in September and will spend 5 days in Barcelona and about 5 days in Seville. I am looking for recommendaions of unique villages to visit as a side/day trip from those locations. Thanks, Susan

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Planning to use public transportation but will consider renting a car if we find that is the only way to get to best villages.

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Planning to use public transportation but will consider renting a car if we find that is the only way to get to best villages.

In that case, I would suggest Rupit, Queralbs, Castellfollit de la Roca, Miravet, or Cadaqués for unique villages nearish to Barcelona.