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Cheap buses from Barcelona to France

I've seen the FlixBus, and City2City, and MeinFernBus in Germany that travel between German cities and beyond for very reasonable prices - like 8 Euros from Munchen to Frankfurt. Is there a bus service like that in Spain that we can use to get from Barcelona to Toulouse or really, anywhere in the south of France?

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There are many bus companies within Spain, but for international trips, start with www.eurolines.com. The fastest trains from Barcelona to Toulouse take about 4 hours with a connection at Narbonne, or one afternoon departure is faster and direct. Train tickets are cheaper when you buy them early, up to 4 months in advance.