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Where to Begin Travels -- Barcelona or Taull

We anticipate returning to Barcelona (our 4Runner is parked here) on 22 August about mid-morning. At this time of year, taking in weather & tourist (local & foreign) where should we start our 89 driving tour:
Option 1 -- Barcelona for 10 nights and then Montserrat/Andorra/Taull/Tarragona
Option 2 -- Barcelona & drive to Montserrat 1n/Andorra 1n/Taull 3n/Barcelona 10 n/Tarragona 2n & continue travels & fly home about 16 Nov from Madrid
Does it really make a difference if we start Barcelona exploring on August 22 or August 27?

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