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Possible Itinerary in May with Barcelona day trips.

Thinking of getting away for 2 weeks to include mainly staying in Barcelona, perhaps breaking it up mid-trip with a few nights in Madrid via train. We would like to do day-trips from Barcelona, like Tarragona, Monserrat, Girona. Looking for suggestions for day-trips and why. We have a very hectic 50-day trip in the fall training through Europe, so looking for a little bit more relaxed trip in the Spring.

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From Barcelona, there are many different day trips for many different interests of many different people. A selection of my favorites:

Ancient history
Tarragona
Empúries

Moorish history
Zaragoza
Girona

Medieval History
Poblet Monastery
Vic

Hiking
Camino de Ronda
Vall de Núria

Beach Day
Sitges
Tossa de Mar

Small towns:
Rupit
Besalú