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Pilgrimage to Montserrat and Manresa in one day

While visiting Barcelona with my wife this coming September for few days, I would like to pay visit to Montserrat and Manresa in one day preferably with guided tour. But I couldn't find such a tour! The ones I found are all for Monserrat without Manresa. Should we go on our own? In this case should we take the train, coach or rent a car?

Thanks!

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