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Portugal to Spain

Hey all, I’m considering trying to do both countries in 2 weeks. Trying to determine the best way to connect the two. Anyone have any experience with the bus that runs from Faro to Seville?

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Alsa plies the route (and maybe other companies). It takes about 3 hours and it is quite reliable (traffic is not much of an issue in those parts).
However, a 2-week itinerary that combines Spain and Portugal perhaps should not include the Algarve as a top priority? There are flights from Lisbon to Seville that can help you skip that area entirely. It depends what you are trying to do: Lisbon + Algarve + Andalucía can fit in 2 weeks, but if you want to see more of Spain than just Andalucía, then skip the Algarve.