@bherrington47 - Inishmore is a small place (that is, not a ton of infrastructure); choices for accommodations, food, etc. are limited, and you would be booking pretty late (but most people just come as day-trippers, so that's on your side). That said, I just did a quick peek at booking.com and airbnb.com, I do see a few options (literally, just a few, so you won't be able to be too picky). I stayed at a different B&B, so am not familiar with those that are available; you should take a look and see if they align with your needs/tastes/budget.
I see no need for a car once you reach Galway (unless you have plans to see something outside town). Galway itself is absolutely walkable. The little plane flies from their own airstrip outside of town, you buy a ticket to/from the airstrip on their own bus when you book your air ticket (ask); IIRC it was around 10€ for the bus (it's a vintage "heritage" bus). So once you reach Galway, no need for a car (no need to pay for one or worry about parking, either). When you're done with Inishmore, you can catch a bus or train back to Dublin (no reason to drive).
Your updated schedule looks fine to me. You could spend a full day in Galway if you want to, or you could just use Galway for sleeping on the way in and out to Inishmore. You could spend a day in Galway either before or after your side-trip out to Inishmore. Or you could spend that day somewhere else along your route if you short-changed anyplace.
Honestly, I'm not sure you really need a guided tour of Inishmore; we spent 3 days/2 nights (part of the first and 3rd day, all of the 2nd day) there and managed well enough on our own with a guidebook (we are not big on guided tours).
I don't believe there are cars to rent on the island. There are E-bikes. That's what we rented, it helped a lot (there are hills and it is often windy). There are "taxis" of various kinds (horse-drawn carts and cars). The airstrip folks drop you at your accommodations in a van after you arrive. Expect to do more than a little walking (and biking if you're up for it) as you explore the island. We loved it - it was a highlight of our trip.
Tip: When you book the flight, and when you check in for the flight at their airstrip, ask if you can get the right front seat (it's the copilot seat). Some lucky person gets to sit there, might as well ask for it...best views you'll ever have from an airplane if you're lucky enough to get it (flight is less than 10 minutes, so enjoy it while you can). Hope that helps.