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Car Rental in Santorini

We'll be in Santorini for 3 days, arriving at and departing from the Athinios port, via ferry. Any recommendations for a good rental car company? And, any insights as to whether it would be best to rent a car at the port as soon as we arrive or to get one for just two of the three days we're there, if it's possible to pick up a car in Fira and drop it off at the Athinios port?

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