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10 day Road Trip Marseille to Barcelona fly home Toulouse

10 day Road Trip: Marseille to Barcelona fly home from Toulouse. Going via Arles, Montpellier, Collioure, Barcelona, back up the coast, Carcassonne, ending in Toulouse to fly home. Planning 3 nights in Barcelona Oct. 1-4. Other night stays & towns are negotiable, preferring 2 night stays when feasible. Recommendations welcome! We will have already been in Provence before this drive.

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Girona, Spain would make a great stay for 2-3 nights.
Besalu is also fascinating and is just 30 minutes from Girona.