Well, definitely see the Treasure Room in the British Library.
Bletchley is definitely worth the effort. I thought I’d spend 2 hours there. Spent 4. Very well done!
Have you seen the Crystal Palace Dinosaurs?
Toured Wimbledon?
The Hunterian Museum is interesting and afterwards be sure to visit the Seven Star pub. 5 minute walk.
Cozy pub, fab pub cat and tasty pasta dishes.
Walking along the Thames River Path is enjoyable. So is strolling along the Regents Canal Path. Watching the narrow boats, dog walkers…
If you want to get out of London proper there’s the Parkland Trail. I enjoyed a meander on it from Finsbury Park to Crouch End.
Enjoying the massive Richmond Park and seeing the fallow deer is a great excursion if weather is good. Then buy cheese at Teddington Cheese if you exit the park by where the Royal Star and Garter Home is located. If timing is right u could have a pint at the Victorian Inn ( no food there) and or go into the pleasant Books on The Rise. 15 -20 minute walk to Richmond Station to board an Underground train or SW train back to Covent Garden. Allot 60 minutes.
Definitely search out street markets. Brick Lane, Columbia Road Flower Market, Broadway Market in Hackney, and Maltby Market.
Must say check out Spitalfields. Depending when in the Fall you are traveling ( I go in November ) you can find Xmas ornaments, stocking stuffers and boxes of Xmas cards.
If LP lovers or if you know an afficiado and your dates coincide; https://oldspitalfieldsmarket.com/events/vinyl-market
Been going to London since Nixon was President. Never fails to provide new sites to explore and enjoy.
Enjoy.