I haven't visited Plymouth but as I think I mentioned maybe in an earlier thread you had on Devon and Cornwall that I did a Road Scholar program that stayed in Falmouth. I really enjoyed that town but I'm not sure about parking if you are driving. I stayed at a large, old seafront hotel.
As far as things I enjoyed, I, too, loved Lost Gardens of Heligan. Didn't do the Eden Project but we did a china clay mine tour at Wheal Martyn just outside St Austell. I'm not big on mine tours but it was more interesting than the Levant or Geevor Tin Mine we also did. (Geevor is also on the Rick Steves Villages of Southern England tour).
I liked St Michaels Mount but it is pretty steep and slippery up to the front door of the house. The tides here are interesting and it was cool to watch the walkway out to the isle be covered with water and then watch it recede.
I thought the Iron Age Chysauster Ancient Village was quite interesting. It also has a neolithic Fogou which is an underground passage.
https://en.wikipedia.org/wiki/Chysauster_Ancient_Village
I didn't much care for St Ives but it was school half term and it was jammed with families so more people around than I like. I did like Mevagissey as well as St Mawes (you can take a ferry across from Falmouth), Charlestown, Fowey and Boscastle. I've visited Port Isaac twice and while I was excited the first time because I'm a Doc Martin fan, really, it's terribly crowded and you can see everything in about an hour.